Have you tried unwound 4th strings? Aquila Reds are really good, although they are a bit fatter than the average string, so a wider nut slot to compensate would help if you researched and committed to a low G Red string. I think according to the mixed reviews, it's a gamble on whether it breaks or not if you don't widen the nut slot, but the sound quality is something I think a lot of people enjoy. It may be too "flappy" for C tuning - D works better for the tension and sound. I heard Worth makes unwound 4ths as well.
La Bella makes a great wound 4th in my opinion - I have La Bella gold basses on my classical guitar and the response is warm and nice. Tension is average, and no string squeak! If you wanted a sharp response from your bass string though, it probably isn't a good choice, because there are reviews saying the bass is a bit too soft, even to the point where some may say it is dead? I don't think so!
If not these, Southcoast is the best and safest option (even skipping Aquila and La Bella) because you can talk to Dirk, and although he may be a little swamped with incoming arrivals and cataloging new products, he'll be the best choice in helping you find your fit. You should read this link from their website first, though - Dirk will probably direct it to you eventually xD (
http://www.southcoastukes.com/tunings.htm)
Southcoast string sets page (scroll through the reading):
http://www.southcoastukes.com/string sets.htm
Also, if you have the time, read the other links about tuning and strings on his website. The accumulation of luthier and musical knowledge on his website is totally relevant to how we see and play the ukulele today!
All in all, I would just ask myself: "what kind of sound do I want from my ukulele?" and then just start from there. Good luck!